Photonic Materials & Devices

Dimensionality plays a crucial role in long-range dipole-dipole interactions (DDIs). We demonstrate that a resonant nanophotonic structure modifies the apparent dimensionality in an interacting ensemble of emitters, as revealed by population decay dynamics. Our measurements on a dense ensemble of interacting quantum emitters in a resonant nanophotonic structure with long-range DDIs reveal an effective dimensionality reduction to ¯d=2.20(12), despite the emitters being distributed in 3D. This contrasts with the homogeneous environment, where the apparent dimension is ¯d=3.00. Our work presents a promising avenue to manipulate dimensionality in an ensemble of interacting emitters.

Nonreciprocal gyrotropic materials have attracted significant interest recently in material physics, nanophotonics, and topological physics. Most of the well-known nonreciprocal materials, however, only show nonreciprocity under a strong external magnetic field and within a small segment of the electromagnetic spectrum. Here, through first-principles density-functional theory calculations, we show that due to strong spin-orbit coupling manganese-bismuth (MnBi) exhibits nonreciprocity without any external magnetic field and a large gyrotropy in a broadband long-wavelength infrared regime. Further, we design a multilayer structure based on MnBi to obtain a maximum degree of spin-polarized thermal emission at 7 µm. The connection established here between large gyrotropy and the spin-polarized thermal emission points to the potential use of MnBi to develop spin-controlled thermal photonics platforms.

The engineering of the spatial and temporal properties of both the electric permittivity and the refractive index of materials is at the core of photonics. When vanishing to zero, those two variables provide efficient knobs to control light–matter interactions. This Perspective aims at providing an overview of the state of the art and the challenges in emerging research areas where the use of near-zero refractive index and hyperbolic metamaterials is pivotal, in particular, light and thermal emission, nonlinear optics, sensing applications, and time-varying photonics.

Spinning thermal radiation is a unique phenomenon observed in condensed astronomical objects, including the Wolf-Rayet star EZ-CMa and the red degenerate star G99-47, due to the existence of strong magnetic fields. Here, by designing symmetry-broken metasurfaces, we demonstrate that spinning thermal radiation with a nonvanishing optical helicity can be realized even without applying a magnetic field. We design nonvanishing optical helicity by engineering a dispersionless band that emits omnidirectional spinning thermal radiation, where our design reaches 39% of the fundamental limit. Our results firmly suggest that metasurfaces can impart spin coherence in the incoherent radiation excited by thermal fluctuations. The symmetry-based design strategy also provides a general pathway for controlling thermal radiation in its temporal and spin coherence.

Engineering symmetries in nanostructures and metasurfaces provides a new paradigm to control incoherent heat radiation for applications in energy conversion, thermal sources, infrared imaging, and radiative cooling.

The fluctuational electrodynamic investigation of thermal radiation from nonequilibrium or nonisothermal bodies remains largely unexplored because it necessarily requires volume integration over the fluctuating currents inside the emitter, which quickly becomes computationally intractable. Here, we put forth a formalism combining fast calculations based on modal expansion and fluctuational electrodynamics to accelerate research at this frontier. We employ our formalism on a sample problem: a long silica wire held under temperature gradient within its cross section. We discover that the far-field thermal emission carries a nonzero spin, which is constant in direction and sign, and interestingly, is transverse to the direction of the power flow. We clearly establish the origin of this transverse spin as arising from the nonequilibrium intermixing of the cylindrical modes of the wire, and not from any previously studied or intuitively expected origins such as chiral or nonisotropic materials and geometries, magnetic materials or fields, and mechanical rotations. This finding of nonequilibrium spin texture of emitted heat radiation can prove useful for advancing the noninvasive thermal metrology or infrared-imaging techniques.

Thermal radiation is traditionally an incoherent radiative signal, where the radiated heat is highly unpolarized, spectrally broad, and omnidirectional. The recent extensive interests in thermal photonics focus on tailoring the temporal coherence (spectrum) and spatial coherence (directivity) of thermal radiation. Here, we investigate the photon spin characteristics of the radiation excited by thermal fluctuations using a symmetrybroken metasurface. Utilizing spin-polarized angle-resolved thermal emission spectroscopy (SPARTES), we explicitly show when both mirror- and inversion- symmetries are broken, the summation of spin-angular momentum projected on wavevectors, namely the optical helicity, can be non-vanishing even without applying a magnetic field. We find the photon spin and the energy-momentum dispersion of thermal radiation can be effectively tailored through symmetry engineering. Our results firmly suggest the symmetry-based strategy provides a general pathway for comprehensively controlling the temporal, spatial, and especially spin coherence of thermal radiation.

A powerful result of topological band theory is that nontrivial phases manifest obstructions to constructing
localized Wannier functions. In Chern insulators, it is impossible to construct Wannier functions that respect
translational symmetry in both directions. Similarly, Wannier functions that respect time-reversal symmetry
cannot be formed in quantum spin Hall insulators. This molecular orbital interpretation of topology has been
enlightening and was recently extended to topological crystalline insulators which include obstructions tied to
space-group symmetries. In this paper, we introduce a class of two-dimensional topological materials known
as optical N-insulators that possess obstructions to construct localized molecular polarizabilities. The optical
N-invariant N ∈ Z is the winding number of the atomistic susceptibility tensor χ and counts the number of
singularities in the electromagnetic linear response theory. We decipher these singularities by analyzing the
optical band structure of the material—the eigenvectors of the susceptibility tensor—which constitutes the
collection of optical Bloch functions. The localized basis of these eigenvectors is optical Wannier functions
which characterize the molecular polarizabilities at different lattice sites. We prove that in a nontrivial optical
phase N = 0, such a localized polarization basis is impossible to construct. Utilizing the mathematical machinery
of K theory, these optical N-phases are refined further to account for the underlying crystalline symmetries of
the material, generating a complete classification of the topological electromagnetic phase of matter.

Germanium is typically used for solid-state electronics, fiber-optics, and infrared applications, due to its semiconducting behavior at optical and infrared wavelengths. In contrast, here we show that the germanium displays metallic nature and supports propagating surface plasmons in the deep ultraviolet (DUV) wavelengths, that is typically not possible to achieve with conventional plasmonic metals such as gold, silver, and aluminum. We measure the photonic band spectrum and distinguish the plasmonic excitation modes: bulk plasmons, surface plasmons, and Cherenkov radiation using a momentum-resolved electron energy loss spectroscopy. The observed spectrum is validated through the macroscopic electrodynamic electron energy loss theory and first-principles density functional theory calculations. In the DUV regime, intraband transitions of valence electrons dominate over the interband transitions, resulting in the observed highly dispersive surface plasmons. We further employ these surface plasmons in germanium to design a DUV radiation source based on the Smith-Purcell effect. Our work opens a new frontier of DUV plasmonics to enable the development of DUV devices such as metasurfaces, detectors, and light sources based on plasmonic germanium thin films.

Spontaneous emission of quantum emitters can be enhanced by increasing the local density of optical states, whereas engineering dipole–dipole interactions requires modifying the two-point spectral density function. Here, we experimentally demonstrate long-range dipole–dipole interactions (DDIs) mediated by surface lattice resonances in a plasmonic nanoparticle lattice. Using angle-resolved spectral measurements and fluorescence lifetime studies, we show that unique nanophotonic modes mediate long-range DDI between donor and acceptor molecules. We observe significant and persistent DDI strengths for a range of densities that map to ∼800 nm mean nearest-neighbor separation distance between donor and acceptor dipoles, a factor of ∼100 larger than free space. Our results pave the way to engineer and control long-range DDIs between an ensemble of emitters at room temperature.

We numerically demonstrate that a planar slab made of magnetic Weyl semimetal (a class of topological materials) can emit high-purity circularly polarized (CP) thermal radiation over a broad mid- and long-wave infrared wavelength range for a significant portion of its emission solid angle. This effect fundamentally arises from the strong infrared gyrotropy or nonreciprocity of these materials, which primarily depends on the momentum separation between Weyl nodes in the band structure. We clarify the dependence of this effect on the underlying physical parameters and highlight that the spectral bandwidth of CP thermal emission increases with increasing momentum separation between the Weyl nodes. We also demonstrate, using the recently developed thermal discrete dipole approximation (TDDA) computational method, that finite-size bodies of magnetic Weyl semimetals can emit spectrally broadband CP thermal light, albeit over smaller portion of the emission solid angle compared to the planar slabs. Our work identifies unique fundamental and technological prospects of magnetic Weyl semimetals for engineering thermal radiation and designing efficient CP light sources.

Spin and orbital angular momentum of light plays a central role in quantum nanophotonics as well as topological electrodynamics. Here, we show that the thermal radiation from finite-size bodies comprising nonreciprocal magneto-optical materials can exert a spin torque even in global thermal equilibrium. Moving beyond the paradigm of near-field heat transfer, we calculate near-field radiative angular momentum transfer between finite-size nonreciprocal objects by combining Rytov's fluctuational electrodynamics with the theory of optical angular momentum. We prove that a single magneto-optical cubic particle in nonequilibrium with its surroundings experiences a torque in the presence of an applied magnetic field (T-symmetry breaking). Furthermore, even in global thermal equilibrium, two particles with misaligned gyrotropy axes experience equal-magnitude torques with opposite signs which tend to align their gyrotropy axes parallel to each other. Our results are universally applicable to semiconductors like InSb (magnetoplasmas) as well as Weyl semimetals which exhibit the anomalous Hall effect (gyrotropic) at infrared frequencies. Our work paves the way towards near-field angular momentum transfer mediated by thermal fluctuations for nanoscale devices.

Extreme skin depth engineering (e-skid) can be applied to integratedphotonics to manipulate the evanescent field of a waveguide. Here wedemonstrate that e-skid can be implemented in two directions in order todeterministically engineer the evanescent wave allowing for denseintegration with enhanced functionalities. In particular, by increasingthe skin depth, we enable the creation of two-dimensional (2D) e-skiddirectional couplers with large gaps and operational bandwidth. Here weexperimentally validate 2D e-skid for integrated photonics in acomplementary metal--oxide semiconductor (CMOS) photonics foundry anddemonstrate strong coupling with a gap of 1.44 {\textmu}m.

Current crowding at bends of superconducting nanowire single-photon detector (SNSPD) is one of the main factors limiting the performance of meander-style detectors with large filling factors. In this paper, we propose a new concept to reduce the influence of the current crowding effect, a so-called variable thickness SNSPD, which is composed of two regions with different thicknesses. A larger thickness of bends in comparison to the thickness of straight nanowire sections locally reduces the current density and reduces the suppression of the critical current caused by current crowding. This allows variable thickness SNSPD to have a higher critical current, an improved detection efficiency, and decreased dark count rate in comparison with a standard uniform thickness SNSPD with an identical geometry and film quality.

Abstract The strong electric and magnetic resonances in dielectric subwavelength structures have enabled unique opportunities for efficient manipulation of light–matter interactions. Besides, the dramatic enhancement of nonlinear light–matter interactions near so-called bound states in the continuum (BICs) has recently attracted enormous attention due to potential advancements. However, the experimental realizations and the applications of high-Q factor resonances in dielectric resonances in the visible have thus far been considerably limited. In this work, the interplay of electric and magnetic dipoles in arrays of dielectric nanoresonators is explored. The experimental realization of high-Q factor resonances in the visible through the collective diffractive coupling of electric and magnetic dipoles is reported. It is also shown that coupling the Rayleigh anomaly of the array with the dipoles of the individual nanoresonators can result in the formation of different types of BICs. The resonances in the visible regime is utilized to achieve lasing action at room temperature with high spatial directionality and low threshold. Finally, multi-mode, directional lasing is experimentally demonstrated and the BIC-assisted lasing mode engineering in arrays of dielectric nanoresonators is studied. It is believed that the results enable a new range of applications in flat photonics through realizing on-chip controllable single and multi-wavelength micro-lasers.

A chiral absorber of light can emit spin-polarized (circularly polarized) thermal radiation based on Kirchhoff’s law which equates spin-resolved emissivity with spin-resolved absorptivity for reciprocal media at thermal equilibrium. No such law is known for nonreciprocal media. In this work, we discover three spin-resolved Kirchhoff’s laws of thermal radiation applicable for both reciprocal and nonreciprocal planar media. In particular, these laws are applicable to multi-layered or composite slabs of generic bianisotropic material classes which include (uniaxial or biaxial) birefringent crystals, (gyrotropic) Weyl semimetals, magnetized semiconductors, plasmas, ferromagnets and ferrites, (magnetoelectric) topological insulators, metamaterials and multiferroic media. We also propose an experiment to verify these laws using a single system of doped indium antimonide (InSb) thin film in an external magnetic field. Furthermore, we reveal a surprising result that the planar slabs of all these material classes can emit partially circularly polarized thermal light without requiring any surface patterning, and identify planar configurations which can experience nontrivial thermal optomechanical forces and torques upon thermal emission into the external environment at lower temperature (nonequilibrium). Our work also provides a new fundamental insight of detailed balance of angular momentum (in addition to energy) of equilibrium thermal radiation, and paves the way for practical functionalities based on thermal radiation using nonreciprocal bianisotropic materials.

Chern-Simons theories have been very successful in explaining integer and fractional quantum Hall phases of matter, topological insulators, and Weyl semimetals. However, it remains an open question as to whether Chern-Simons theories can be adapted to topological photonics. We develop a viscous Maxwell-Chern-Simons theory to capture the fundamental physics of a topological electromagnetic phase of matter. We show the existence of a unique spin-1 skyrmion in the viscous Hall fluid arising from a photonic Zeeman interaction in momentum space. Our work bridges the gap between electromagnetic and condensed matter topological physics while also demonstrating the central role of photon spin-1 quantization in identifying new phases of matter.

Controlling and detecting thermal radiation is of vital importance for varied applications ranging from energy conversion systems and nanoscale information processing devices to infrared imaging, spectroscopy, and sensing. We review the field of high-temperature thermal photonics, which aims to control the spectrum, polarization, tunability, switchability, and directionality of heat radiation from engineered materials in extreme environments. We summarize the candidate materials that are being pursued by the community that have simultaneous polaritonic/plasmonic properties as well as high-temperature stability. We also provide a detailed discussion of common photonic platforms, including metagratings, photonic crystals, and metamaterials used for thermal emission engineering. We review broad applications, including thermophotovoltaics, high-temperature radiative cooling, thermal radiation sources, and noisy nanoscale thermal devices. By providing an overview of the recent achievements in this field, we hope this review can accelerate progress to overcome major outstanding problems in modern thermal engineering.

Over the past decade, topology has emerged as a major branch in broad areas of physics, from atomic lattices to condensed matter. In particular, topology has received significant attention in photonics because light waves can serve as a platform to investigate nontrivial bulk and edge physics with the aid of carefully engineered photonic crystals and metamaterials. Simultaneously, photonics provides enriched physics that arises from spin-1 vectorial electromagnetic fields. Here, we review recent progress in the growing field of topological photonics in three parts. The first part is dedicated to the basics of topological band theory and introduces various two-dimensional topological phases. The second part reviews three-dimensional topological phases and numerous approaches to achieve them in photonics. Last, we present recently emerging fields in topological photonics that have not yet been reviewed. This part includes topological degeneracies in nonzero dimensions, unidirectional Maxwellian spin waves, higher-order photonic topological phases, and stacking of photonic crystals to attain layer pseudospin. In addition to the various approaches for realizing photonic topological phases, we also discuss the interaction between light and topological matter and the efforts towards practical applications of topological photonics.

Superconducting nanowire single-photon detectors have emerged as a promising technology for quantum metrology from the mid-infrared to ultraviolet frequencies. Despite recent experimental successes, a predictive model to describe the detection event in these detectors is needed to optimize the detection metrics. Here, we propose a probabilistic criterion for single-photon detection based on single-vortex (flux quanta) crossing the width of the nanowire. Our model makes a connection between the dark counts and photon counts near the detection threshold. The finite-difference calculations demonstrate that a change in the bias current distribution as a result of the photon absorption significantly increases the probability of single-vortex crossing even if the vortex potential barrier has not vanished completely. We estimate the instrument response function and show that the timing uncertainty of this vortex tunneling process corresponds to a fundamental limit in timing jitter of the click event. We demonstrate a trade-space between this intrinsic (quantum) timing jitter, quantum efficiency, and dark count rate in TaN, WSi, and NbN superconducting nanowires at different experimental conditions. Our detection model can also explain the experimental observation of exponential decrease in the quantum efficiency of SNSPDs at lower energies. This leads to a pulse-width dependency in the quantum efficiency, and it can be further used as an experimental test to compare across different detection models.